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Evasion of Elemental Mercury from a Boreal Peatland Suppressed by Long-Term Sulfate Addition
JournalArticle (Originalarbeit in einer wissenschaftlichen Zeitschrift)
 
ID 2821781
Author(s) Fritsche, Johannes; Osterwader, Stefan; Nilsson, Mats B.; Sagerfors, Jorgen; Akerblom, Staffan; Bishop, Kevin; Alewell, Christine
Author(s) at UniBasel Osterwalder, Stefan
Alewell, Christine
Year 2014
Title Evasion of Elemental Mercury from a Boreal Peatland Suppressed by Long-Term Sulfate Addition
Journal Environmental science & technology letters
Volume 1
Number 10
Pages / Article-Number 421-425
Keywords Atmospheric mercury, air-surface exchange, dynamic flux chamber, sulfur deposition, oligotrophic mire, wetlands, background soils
Abstract

We investigated the evasion of TGM (total gaseous mercury) from
experimental plots on a boreal peatland that had been exposed for 15 years to
different combinations of atmospheric sulfur (S) and nitrogen (N) deposition as well
as greenhouse treatments simulating climate change. Shaded dynamic flux chamber
measurements during the summer in 2009 showed emission of TGM to the
atmosphere from most of the treated plots (0.7 ± 0.94 ng m−2 h−1). However, TGM
exchange rates were significantly lower, occasionally indicating Hg uptake, on plots
subjected to S addition at rates of 20 kg ha−1 year−1. Enhanced nitrogen deposition
and greenhouse treatment had no significant effect on TGM fluxes. We hypothesize
that the lower Hg evasion from the sulfur-treated plots is related to either earlier Hg
evasion or Hg binding to S in organic matter, making Hg less susceptible to
volatilization and more prone to transport in runoff.

Publisher ACS
ISSN/ISBN 2328-8930
URL http://pubs.acs.org/doi/abs/10.1021/ez500223a
edoc-URL http://edoc.unibas.ch/dok/A6337735
Full Text on edoc No
Digital Object Identifier DOI 10.1021/ez500223a
ISI-Number WOS:000350831600008
Document type (ISI) Article
 
   

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